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Outlook For Ios Adds Contacts Support Eightwone 1  Now you will need to press the Add Mail Account option so you can begin configuring your mail account On the next screen you will need to fill your Name, email Address, Password and few words for the mail account Description Once you are done with these configurations please click the Next button so you can proceed with the configuration further Here are steps about how to set up multiple Outlook accounts on an iPhone Launch the Settings App on your iPhone Tap on Mail, Connects, Calendars Tap on Add Account Tap on Outlookcom Enter your Outlookcom username and password and then tap Next in the upper right hand corner Choose the services you'd like to enable and sync with Outlook and then tap Save Outlook iphone sync settings